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Removal of lead(II) by nanofiltration-ranged thin film nanocomposite membrane incorporated UiO-66-NH2: comparative removal performance between hydraulic-driven and osmotic-driven membrane process

Backgrounds: Contamination of heavy metals has attracted great attention in scientific community in which membrane technology by using thin film composite (TFC) membrane has shown a great potential for treating contaminated water. Methods: This study aimed to develop thin film nanocomposite (TFN) in...

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Main Authors: Abdullah, Norfadhilatuladha, Yusof, Norhaniza, Lau, Woei Jye, Jaafar, Juhana, Misdan, Nurasyikin, Ismail, Ahmad Fauzi
Format: Article
Published: Taiwan Institute of Chemical Engineers 2021
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TP Chemical technology
Online Access:http://eprints.utm.my/id/eprint/94652/
http://dx.doi.org/10.1016/j.jtice.2021.08.047
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spelling my.utm.946522022-03-31T15:51:55Z http://eprints.utm.my/id/eprint/94652/ Removal of lead(II) by nanofiltration-ranged thin film nanocomposite membrane incorporated UiO-66-NH2: comparative removal performance between hydraulic-driven and osmotic-driven membrane process Abdullah, Norfadhilatuladha Yusof, Norhaniza Lau, Woei Jye Jaafar, Juhana Misdan, Nurasyikin Ismail, Ahmad Fauzi TP Chemical technology Backgrounds: Contamination of heavy metals has attracted great attention in scientific community in which membrane technology by using thin film composite (TFC) membrane has shown a great potential for treating contaminated water. Methods: This study aimed to develop thin film nanocomposite (TFN) incorporated with different loading of water-stable UiO-66-NH2 and its comparative performance for removing lead (Pb) from water by hydraulic-driven nanofiltration (NF) and osmotic-driven forward osmosis (FO) process. Significant findings: In terms of membrane performance for Pb(II) removal by NF process, increasing Pb(II) initial concentration and the presence of multi-valent ions; cadmium (Cd)/nickel (Ni) decreased Pb(II) rejection for TFN/UiO-66-NH2. Interestingly, under the forward osmosis (FO) process, Pb(II) initial concentration and presence of multi-valent ions (Cd/Ni) did not influence the rejection of Pb(II) in which 99% rejection was achieved for all membranes. TFN/UiO-66-NH2 offered higher FO water flux as compared to the control membrane. In comparison to NF process using the same membrane, the rejection via FO process was 30% more efficient. Results from this study has proven that the incorporation of UiO-66-NH2 improved the properties of TFN membranes making it suitable to be used for water/wastewater treatment and FO can be as another alternative technique for heavy metals removal. Taiwan Institute of Chemical Engineers 2021-11 Article PeerReviewed Abdullah, Norfadhilatuladha and Yusof, Norhaniza and Lau, Woei Jye and Jaafar, Juhana and Misdan, Nurasyikin and Ismail, Ahmad Fauzi (2021) Removal of lead(II) by nanofiltration-ranged thin film nanocomposite membrane incorporated UiO-66-NH2: comparative removal performance between hydraulic-driven and osmotic-driven membrane process. Journal of the Taiwan Institute of Chemical Engineers, 128 . pp. 354-369. ISSN 1876-1070 http://dx.doi.org/10.1016/j.jtice.2021.08.047 DOI:10.1016/j.jtice.2021.08.047
institution Universiti Teknologi Malaysia
building UTM Library
collection Institutional Repository
continent Asia
country Malaysia
content_provider Universiti Teknologi Malaysia
content_source UTM Institutional Repository
url_provider http://eprints.utm.my/
topic TP Chemical technology
spellingShingle TP Chemical technology
Abdullah, Norfadhilatuladha
Yusof, Norhaniza
Lau, Woei Jye
Jaafar, Juhana
Misdan, Nurasyikin
Ismail, Ahmad Fauzi
Removal of lead(II) by nanofiltration-ranged thin film nanocomposite membrane incorporated UiO-66-NH2: comparative removal performance between hydraulic-driven and osmotic-driven membrane process
description Backgrounds: Contamination of heavy metals has attracted great attention in scientific community in which membrane technology by using thin film composite (TFC) membrane has shown a great potential for treating contaminated water. Methods: This study aimed to develop thin film nanocomposite (TFN) incorporated with different loading of water-stable UiO-66-NH2 and its comparative performance for removing lead (Pb) from water by hydraulic-driven nanofiltration (NF) and osmotic-driven forward osmosis (FO) process. Significant findings: In terms of membrane performance for Pb(II) removal by NF process, increasing Pb(II) initial concentration and the presence of multi-valent ions; cadmium (Cd)/nickel (Ni) decreased Pb(II) rejection for TFN/UiO-66-NH2. Interestingly, under the forward osmosis (FO) process, Pb(II) initial concentration and presence of multi-valent ions (Cd/Ni) did not influence the rejection of Pb(II) in which 99% rejection was achieved for all membranes. TFN/UiO-66-NH2 offered higher FO water flux as compared to the control membrane. In comparison to NF process using the same membrane, the rejection via FO process was 30% more efficient. Results from this study has proven that the incorporation of UiO-66-NH2 improved the properties of TFN membranes making it suitable to be used for water/wastewater treatment and FO can be as another alternative technique for heavy metals removal.
format Article
author Abdullah, Norfadhilatuladha
Yusof, Norhaniza
Lau, Woei Jye
Jaafar, Juhana
Misdan, Nurasyikin
Ismail, Ahmad Fauzi
author_facet Abdullah, Norfadhilatuladha
Yusof, Norhaniza
Lau, Woei Jye
Jaafar, Juhana
Misdan, Nurasyikin
Ismail, Ahmad Fauzi
author_sort Abdullah, Norfadhilatuladha
title Removal of lead(II) by nanofiltration-ranged thin film nanocomposite membrane incorporated UiO-66-NH2: comparative removal performance between hydraulic-driven and osmotic-driven membrane process
title_short Removal of lead(II) by nanofiltration-ranged thin film nanocomposite membrane incorporated UiO-66-NH2: comparative removal performance between hydraulic-driven and osmotic-driven membrane process
title_full Removal of lead(II) by nanofiltration-ranged thin film nanocomposite membrane incorporated UiO-66-NH2: comparative removal performance between hydraulic-driven and osmotic-driven membrane process
title_fullStr Removal of lead(II) by nanofiltration-ranged thin film nanocomposite membrane incorporated UiO-66-NH2: comparative removal performance between hydraulic-driven and osmotic-driven membrane process
title_full_unstemmed Removal of lead(II) by nanofiltration-ranged thin film nanocomposite membrane incorporated UiO-66-NH2: comparative removal performance between hydraulic-driven and osmotic-driven membrane process
title_sort removal of lead(ii) by nanofiltration-ranged thin film nanocomposite membrane incorporated uio-66-nh2: comparative removal performance between hydraulic-driven and osmotic-driven membrane process
publisher Taiwan Institute of Chemical Engineers
publishDate 2021
url http://eprints.utm.my/id/eprint/94652/
http://dx.doi.org/10.1016/j.jtice.2021.08.047
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score 13.211869

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