Transition of a small-bipolaron gas to a Frohlich polaron in a deformable lattice
The electronic properties of guest Cs atoms in a deformable lattice are investigated at various densities n. Low values of n show optical absorptions of small bipolarons. At intermediate n values, new bands appear in the midinfrared (MIR) and high-frequency regions, which coexist with the small bipo...
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Main Authors: | , , |
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Format: | Article |
Published: |
American Physical Society
2018
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Subjects: | |
Online Access: | http://eprints.utm.my/id/eprint/85472/ http://dx.doi.org/10.1103/PhysRevB.97.155142 |
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Summary: | The electronic properties of guest Cs atoms in a deformable lattice are investigated at various densities n. Low values of n show optical absorptions of small bipolarons. At intermediate n values, new bands appear in the midinfrared (MIR) and high-frequency regions, which coexist with the small bipolaron bands. With a further increase in n, the small bipolaron bands become less discernible and subsequently disappear, resulting in the appearance of a Drude component superimposed on a MIR sideband suggesting a phase transition to a polaronic metal. In this itinerant phase, an approximately twofold mass enhancement is observed. This continuous transition of a gas of small bipolarons to a polaronic metal characterized by a Fröhlich polaron reveals an important part of the complex phase diagram of the metal-insulator transition in a deformable lattice. |
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