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Influence of operating parameters on development of polyethylene oxide-like coatings on the surfaces of polypropylene films by atmospheric pressure cold plasma jet-assisted polymerization to enhance their antifouling properties

In this study, we investigated the deposition of a polyethylene oxide (PEO)-like coating on the surfaces of polypropylene (PP) films via atmospheric pressure cold plasma jet-assisted polymerization using ethylene glycol dimethyl ether as a precursor. The PEO-like coatings were deposited using differ...

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Main Authors:	Pandiyaraj, K. N., ArunKumar, A., Kumar, M. C. Ram, Padmanabhan, P. V. A., Trimukhe, A. M., Deshmukh, R. R., Cools, P., Morent, R., Geyter, N. De, Kumar, V., Gopinath, P., Jaganathan, S. K.
Format:	Article
Published:	Elsevier Ltd 2018
Subjects:	Q Science (General)
Online Access:	http://eprints.utm.my/id/eprint/84625/ http://dx.doi.org/10.1016/j.jpcs.2018.06.007
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spelling	my.utm.846252020-02-27T03:21:10Z http://eprints.utm.my/id/eprint/84625/ Influence of operating parameters on development of polyethylene oxide-like coatings on the surfaces of polypropylene films by atmospheric pressure cold plasma jet-assisted polymerization to enhance their antifouling properties Pandiyaraj, K. N. ArunKumar, A. Kumar, M. C. Ram Padmanabhan, P. V. A. Trimukhe, A. M. Deshmukh, R. R. Cools, P. Morent, R. Geyter, N. De Kumar, V. Gopinath, P. Jaganathan, S. K. Q Science (General) In this study, we investigated the deposition of a polyethylene oxide (PEO)-like coating on the surfaces of polypropylene (PP) films via atmospheric pressure cold plasma jet-assisted polymerization using ethylene glycol dimethyl ether as a precursor. The PEO-like coatings were deposited using different operating parameters (deposition potential and monomer flow rates) and we determined their effects on the film properties, such as the topography, surface chemistry, and surface free energy, based on atomic force microscopy, scanning electron microscopy, transmission electron microscopy, X-ray photoelectron spectroscopy, and contact angle measurements. The interfacial tension between various biological liquids and the PEO-like film surfaces were studied in detail. The antifouling properties of the PEO-like films were examined in vitro, including protein adsorption and platelet adhesion. The results showed that the retention of the PEO-like character and the formation of new functional groups were highly dependent on the operating parameters. Significant changes in the film topography and wettability were obtained by further regulating the plasma operating parameters. All of the PEO-like films had good antifouling properties according to the in vitro analysis results. Elsevier Ltd 2018-12 Article PeerReviewed Pandiyaraj, K. N. and ArunKumar, A. and Kumar, M. C. Ram and Padmanabhan, P. V. A. and Trimukhe, A. M. and Deshmukh, R. R. and Cools, P. and Morent, R. and Geyter, N. De and Kumar, V. and Gopinath, P. and Jaganathan, S. K. (2018) Influence of operating parameters on development of polyethylene oxide-like coatings on the surfaces of polypropylene films by atmospheric pressure cold plasma jet-assisted polymerization to enhance their antifouling properties. Journal of Physics and Chemistry of Solids, 123 . pp. 76-86. ISSN 0022-3697 http://dx.doi.org/10.1016/j.jpcs.2018.06.007
institution	Universiti Teknologi Malaysia
building	UTM Library
collection	Institutional Repository
continent	Asia
country	Malaysia
content_provider	Universiti Teknologi Malaysia
content_source	UTM Institutional Repository
url_provider	http://eprints.utm.my/
topic	Q Science (General)
spellingShingle	Q Science (General) Pandiyaraj, K. N. ArunKumar, A. Kumar, M. C. Ram Padmanabhan, P. V. A. Trimukhe, A. M. Deshmukh, R. R. Cools, P. Morent, R. Geyter, N. De Kumar, V. Gopinath, P. Jaganathan, S. K. Influence of operating parameters on development of polyethylene oxide-like coatings on the surfaces of polypropylene films by atmospheric pressure cold plasma jet-assisted polymerization to enhance their antifouling properties
description	In this study, we investigated the deposition of a polyethylene oxide (PEO)-like coating on the surfaces of polypropylene (PP) films via atmospheric pressure cold plasma jet-assisted polymerization using ethylene glycol dimethyl ether as a precursor. The PEO-like coatings were deposited using different operating parameters (deposition potential and monomer flow rates) and we determined their effects on the film properties, such as the topography, surface chemistry, and surface free energy, based on atomic force microscopy, scanning electron microscopy, transmission electron microscopy, X-ray photoelectron spectroscopy, and contact angle measurements. The interfacial tension between various biological liquids and the PEO-like film surfaces were studied in detail. The antifouling properties of the PEO-like films were examined in vitro, including protein adsorption and platelet adhesion. The results showed that the retention of the PEO-like character and the formation of new functional groups were highly dependent on the operating parameters. Significant changes in the film topography and wettability were obtained by further regulating the plasma operating parameters. All of the PEO-like films had good antifouling properties according to the in vitro analysis results.
format	Article
author	Pandiyaraj, K. N. ArunKumar, A. Kumar, M. C. Ram Padmanabhan, P. V. A. Trimukhe, A. M. Deshmukh, R. R. Cools, P. Morent, R. Geyter, N. De Kumar, V. Gopinath, P. Jaganathan, S. K.
author_facet	Pandiyaraj, K. N. ArunKumar, A. Kumar, M. C. Ram Padmanabhan, P. V. A. Trimukhe, A. M. Deshmukh, R. R. Cools, P. Morent, R. Geyter, N. De Kumar, V. Gopinath, P. Jaganathan, S. K.
author_sort	Pandiyaraj, K. N.
title	Influence of operating parameters on development of polyethylene oxide-like coatings on the surfaces of polypropylene films by atmospheric pressure cold plasma jet-assisted polymerization to enhance their antifouling properties
title_short	Influence of operating parameters on development of polyethylene oxide-like coatings on the surfaces of polypropylene films by atmospheric pressure cold plasma jet-assisted polymerization to enhance their antifouling properties
title_full	Influence of operating parameters on development of polyethylene oxide-like coatings on the surfaces of polypropylene films by atmospheric pressure cold plasma jet-assisted polymerization to enhance their antifouling properties
title_fullStr	Influence of operating parameters on development of polyethylene oxide-like coatings on the surfaces of polypropylene films by atmospheric pressure cold plasma jet-assisted polymerization to enhance their antifouling properties
title_full_unstemmed	Influence of operating parameters on development of polyethylene oxide-like coatings on the surfaces of polypropylene films by atmospheric pressure cold plasma jet-assisted polymerization to enhance their antifouling properties
title_sort	influence of operating parameters on development of polyethylene oxide-like coatings on the surfaces of polypropylene films by atmospheric pressure cold plasma jet-assisted polymerization to enhance their antifouling properties
publisher	Elsevier Ltd
publishDate	2018
url	http://eprints.utm.my/id/eprint/84625/ http://dx.doi.org/10.1016/j.jpcs.2018.06.007
_version_	1662754284421251072
score	13.211869

Influence of operating parameters on development of polyethylene oxide-like coatings on the surfaces of polypropylene films by atmospheric pressure cold plasma jet-assisted polymerization to enhance their antifouling properties

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