Revealing the full potential of CsPbIBr2 perovskite solar cells: advancements towards enhanced performance

Cesium lead iodide bromide (CsPbIBr2) perovskite solar cells (PSCs) have improved stability compared to other perovskite compositions. However, they still face significant challenges due to their poor photovoltaic performance parameters, which limit the devices' power conversion efficiencies (P...

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Main Authors: Hossain M.I., Shahiduzzaman M., Rafij J.H., Tamang A., Akhtaruzzaman M., Hamad A., Uddin J., Amin N., Nunzi J.-M., Taima T.
Other Authors: 57212814509
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Published: Royal Society of Chemistry 2025
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spelling my.uniten.dspace-365012025-03-03T15:42:45Z Revealing the full potential of CsPbIBr2 perovskite solar cells: advancements towards enhanced performance Hossain M.I. Shahiduzzaman M. Rafij J.H. Tamang A. Akhtaruzzaman M. Hamad A. Uddin J. Amin N. Nunzi J.-M. Taima T. 57212814509 55640096500 59141873700 55856822000 57195441001 57196063818 57213630488 7102424614 7005235497 6701678132 Bromine compounds Cesium compounds Conversion efficiency Finite difference time domain method Iodine compounds Layered semiconductors Particle swarm optimization (PSO) Perovskite Perovskite solar cells cesium erythromycin perovskite Device design Finite difference time domains Multi-physics Novel devices Optoelectronics property Particle swarm optimization algorithm Performance Performance parameters Photovoltaic performance Power conversion efficiencies article controlled study electric potential finite element analysis particle swarm optimization solar cell Lead compounds Cesium lead iodide bromide (CsPbIBr2) perovskite solar cells (PSCs) have improved stability compared to other perovskite compositions. However, they still face significant challenges due to their poor photovoltaic performance parameters, which limit the devices' power conversion efficiencies (PCEs). This study proposes a novel device design to tailor the potential of CsPbIBr2 PSCs by improving their optoelectronic properties. An advanced 3D multiphysics approach was rigorously used to investigate the optics and electrical properties of the proposed CsPbIBr2 PSCs. This approach combines finite-difference time-domain (FDTD) and finite element method (FEM) techniques with the particle swarm optimization (PSO) algorithm. The outcome from the adapted numerical approach is in good agreement with the experimental results. The optimized CsPbIBr2 PSC demonstrates a promising power conversion efficiency (PCE) of over 16.4%, associated VOC of 1.53 V, FF of 80.6%, and JSC of 13.4 mA cm?2. Therefore, the potential of CsPbIBr2 perovskites could be further explored with continued research and development in material science and device physics. ? 2024 The Royal Society of Chemistry. Final 2025-03-03T07:42:44Z 2025-03-03T07:42:44Z 2024 Article 10.1039/d4mh00323c 2-s2.0-85197941225 https://www.scopus.com/inward/record.uri?eid=2-s2.0-85197941225&doi=10.1039%2fd4mh00323c&partnerID=40&md5=85eeb1a171d0388e82b26b5b934ea424 https://irepository.uniten.edu.my/handle/123456789/36501 11 18 4329 4337 Royal Society of Chemistry Scopus
institution Universiti Tenaga Nasional
building UNITEN Library
collection Institutional Repository
continent Asia
country Malaysia
content_provider Universiti Tenaga Nasional
content_source UNITEN Institutional Repository
url_provider http://dspace.uniten.edu.my/
topic Bromine compounds
Cesium compounds
Conversion efficiency
Finite difference time domain method
Iodine compounds
Layered semiconductors
Particle swarm optimization (PSO)
Perovskite
Perovskite solar cells
cesium
erythromycin
perovskite
Device design
Finite difference time domains
Multi-physics
Novel devices
Optoelectronics property
Particle swarm optimization algorithm
Performance
Performance parameters
Photovoltaic performance
Power conversion efficiencies
article
controlled study
electric potential
finite element analysis
particle swarm optimization
solar cell
Lead compounds
spellingShingle Bromine compounds
Cesium compounds
Conversion efficiency
Finite difference time domain method
Iodine compounds
Layered semiconductors
Particle swarm optimization (PSO)
Perovskite
Perovskite solar cells
cesium
erythromycin
perovskite
Device design
Finite difference time domains
Multi-physics
Novel devices
Optoelectronics property
Particle swarm optimization algorithm
Performance
Performance parameters
Photovoltaic performance
Power conversion efficiencies
article
controlled study
electric potential
finite element analysis
particle swarm optimization
solar cell
Lead compounds
Hossain M.I.
Shahiduzzaman M.
Rafij J.H.
Tamang A.
Akhtaruzzaman M.
Hamad A.
Uddin J.
Amin N.
Nunzi J.-M.
Taima T.
Revealing the full potential of CsPbIBr2 perovskite solar cells: advancements towards enhanced performance
description Cesium lead iodide bromide (CsPbIBr2) perovskite solar cells (PSCs) have improved stability compared to other perovskite compositions. However, they still face significant challenges due to their poor photovoltaic performance parameters, which limit the devices' power conversion efficiencies (PCEs). This study proposes a novel device design to tailor the potential of CsPbIBr2 PSCs by improving their optoelectronic properties. An advanced 3D multiphysics approach was rigorously used to investigate the optics and electrical properties of the proposed CsPbIBr2 PSCs. This approach combines finite-difference time-domain (FDTD) and finite element method (FEM) techniques with the particle swarm optimization (PSO) algorithm. The outcome from the adapted numerical approach is in good agreement with the experimental results. The optimized CsPbIBr2 PSC demonstrates a promising power conversion efficiency (PCE) of over 16.4%, associated VOC of 1.53 V, FF of 80.6%, and JSC of 13.4 mA cm?2. Therefore, the potential of CsPbIBr2 perovskites could be further explored with continued research and development in material science and device physics. ? 2024 The Royal Society of Chemistry.
author2 57212814509
author_facet 57212814509
Hossain M.I.
Shahiduzzaman M.
Rafij J.H.
Tamang A.
Akhtaruzzaman M.
Hamad A.
Uddin J.
Amin N.
Nunzi J.-M.
Taima T.
format Article
author Hossain M.I.
Shahiduzzaman M.
Rafij J.H.
Tamang A.
Akhtaruzzaman M.
Hamad A.
Uddin J.
Amin N.
Nunzi J.-M.
Taima T.
author_sort Hossain M.I.
title Revealing the full potential of CsPbIBr2 perovskite solar cells: advancements towards enhanced performance
title_short Revealing the full potential of CsPbIBr2 perovskite solar cells: advancements towards enhanced performance
title_full Revealing the full potential of CsPbIBr2 perovskite solar cells: advancements towards enhanced performance
title_fullStr Revealing the full potential of CsPbIBr2 perovskite solar cells: advancements towards enhanced performance
title_full_unstemmed Revealing the full potential of CsPbIBr2 perovskite solar cells: advancements towards enhanced performance
title_sort revealing the full potential of cspbibr2 perovskite solar cells: advancements towards enhanced performance
publisher Royal Society of Chemistry
publishDate 2025
_version_ 1825816274555371520
score 13.244413