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Improving valuable metal ions capturing from spent Li-ion batteries with novel materials and approaches

Rapid growth in the market for batteries is imperative to meet global demand. The lack of economically feasible and environmentally benign recycling process for waste batteries may cause environmental crisis. Taking effective measures could reduce the waste-management challenge and maximize the econ...

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Main Authors:	Aminul Islam, Srimonta Roy, Masud Ali Khan, Pronoy Mondal, Teo, Siow Hwa, Yap, Taufiq Yun Hin, Mohammad Tofayal Ahmed, Tasrina Rabia Choudhury, G. Abdulkreem-Alsultan, Shahjalal Khandaker, Md. Rabiul Awual
Format:	Article
Language:	English English
Published:	Elsevier 2021
Subjects:	TK2896-2985 Production of electricity by direct energy conversion
Online Access:	https://eprints.ums.edu.my/id/eprint/30349/1/Improving%20valuable%20metal%20ions%20capturing%20from%20spent%20Li-ion%20batteries%20with%20novel%20materials%20and%20approaches%20ABSTRACT.pdf https://eprints.ums.edu.my/id/eprint/30349/2/Improving%20valuable%20metal%20ions%20capturing%20from%20spent%20Li-ion%20batteries%20with%20novel%20materials%20and%20approaches%20FULL%20TEXT.pdf https://eprints.ums.edu.my/id/eprint/30349/ https://www.sciencedirect.com/science/article/pii/S0167732221014276?casa_token=tS4uEg5pR0IAAAAA:SHd4z1kST8tk1OipFqfdVnXAYaV3zGV0DOuMm_yqIn42Cqup6l4tk1eqmJFcTHdAsOnKyCXhtOzQ https://doi.org/10.1016/j.molliq.2021.116703
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spelling	my.ums.eprints.303492022-01-10T07:42:08Z https://eprints.ums.edu.my/id/eprint/30349/ Improving valuable metal ions capturing from spent Li-ion batteries with novel materials and approaches Aminul Islam Srimonta Roy Masud Ali Khan Pronoy Mondal Teo, Siow Hwa Yap, Taufiq Yun Hin Mohammad Tofayal Ahmed Tasrina Rabia Choudhury G. Abdulkreem-Alsultan Shahjalal Khandaker Md. Rabiul Awual TK2896-2985 Production of electricity by direct energy conversion Rapid growth in the market for batteries is imperative to meet global demand. The lack of economically feasible and environmentally benign recycling process for waste batteries may cause environmental crisis. Taking effective measures could reduce the waste-management challenge and maximize the economic benefits. In this work, environmentally benign citric acid with the presence of reluctant was used to recover cobalt, manganese, nickel and lithium from waste Lithium Nickel Manganese Cobalt oxide (NCM) batteries. Recovery of Co, Mn, Ni, and Li was optimized by varying the citric acid and H2O2 concentrations, the reaction temperature and duration. The recovery of Co, Mn, Ni, and Li were 87%, 90.5%, 93.5% and 96% respectively under the optimum leaching condition of 1.2 mol/L citric acid, 10 vol% H2O2at 95 for 120 min. Interfacial reaction controlled leaching reaction at low temperature was evident from the results of leaching kinetics with apparent activation energy of 3.75, 10.405.34 and 8.72 kJ mol1 for Co, Mn, Ni and Li, respectively. Importantly, the diffusion controlled leaching reaction was evident from the kinetic and activation energy measurement of leaching. The impact of different chemicals on the environment measured from the Biwer and Heinzle Method (BHM) revealed that the citric acid-assisted leaching process to recover valuable metals from NCM batteries was appeared lower environment impact compare to the other process reported in the literature. The high leaching efficiency and lower impact to the environment provides a novel approach for metal recovery of waste NCM batteries. Elsevier 2021 Article PeerReviewed text en https://eprints.ums.edu.my/id/eprint/30349/1/Improving%20valuable%20metal%20ions%20capturing%20from%20spent%20Li-ion%20batteries%20with%20novel%20materials%20and%20approaches%20ABSTRACT.pdf text en https://eprints.ums.edu.my/id/eprint/30349/2/Improving%20valuable%20metal%20ions%20capturing%20from%20spent%20Li-ion%20batteries%20with%20novel%20materials%20and%20approaches%20FULL%20TEXT.pdf Aminul Islam and Srimonta Roy and Masud Ali Khan and Pronoy Mondal and Teo, Siow Hwa and Yap, Taufiq Yun Hin and Mohammad Tofayal Ahmed and Tasrina Rabia Choudhury and G. Abdulkreem-Alsultan and Shahjalal Khandaker and Md. Rabiul Awual (2021) Improving valuable metal ions capturing from spent Li-ion batteries with novel materials and approaches. Journal of Molecular Liquids, 338. pp. 1-14. ISSN 0167-7322 (P-ISSN) , 1873-3166 (E-ISSN) https://www.sciencedirect.com/science/article/pii/S0167732221014276?casa_token=tS4uEg5pR0IAAAAA:SHd4z1kST8tk1OipFqfdVnXAYaV3zGV0DOuMm_yqIn42Cqup6l4tk1eqmJFcTHdAsOnKyCXhtOzQ https://doi.org/10.1016/j.molliq.2021.116703
institution	Universiti Malaysia Sabah
building	UMS Library
collection	Institutional Repository
continent	Asia
country	Malaysia
content_provider	Universiti Malaysia Sabah
content_source	UMS Institutional Repository
url_provider	http://eprints.ums.edu.my/
language	English English
topic	TK2896-2985 Production of electricity by direct energy conversion
spellingShingle	TK2896-2985 Production of electricity by direct energy conversion Aminul Islam Srimonta Roy Masud Ali Khan Pronoy Mondal Teo, Siow Hwa Yap, Taufiq Yun Hin Mohammad Tofayal Ahmed Tasrina Rabia Choudhury G. Abdulkreem-Alsultan Shahjalal Khandaker Md. Rabiul Awual Improving valuable metal ions capturing from spent Li-ion batteries with novel materials and approaches
description	Rapid growth in the market for batteries is imperative to meet global demand. The lack of economically feasible and environmentally benign recycling process for waste batteries may cause environmental crisis. Taking effective measures could reduce the waste-management challenge and maximize the economic benefits. In this work, environmentally benign citric acid with the presence of reluctant was used to recover cobalt, manganese, nickel and lithium from waste Lithium Nickel Manganese Cobalt oxide (NCM) batteries. Recovery of Co, Mn, Ni, and Li was optimized by varying the citric acid and H2O2 concentrations, the reaction temperature and duration. The recovery of Co, Mn, Ni, and Li were 87%, 90.5%, 93.5% and 96% respectively under the optimum leaching condition of 1.2 mol/L citric acid, 10 vol% H2O2at 95 for 120 min. Interfacial reaction controlled leaching reaction at low temperature was evident from the results of leaching kinetics with apparent activation energy of 3.75, 10.405.34 and 8.72 kJ mol1 for Co, Mn, Ni and Li, respectively. Importantly, the diffusion controlled leaching reaction was evident from the kinetic and activation energy measurement of leaching. The impact of different chemicals on the environment measured from the Biwer and Heinzle Method (BHM) revealed that the citric acid-assisted leaching process to recover valuable metals from NCM batteries was appeared lower environment impact compare to the other process reported in the literature. The high leaching efficiency and lower impact to the environment provides a novel approach for metal recovery of waste NCM batteries.
format	Article
author	Aminul Islam Srimonta Roy Masud Ali Khan Pronoy Mondal Teo, Siow Hwa Yap, Taufiq Yun Hin Mohammad Tofayal Ahmed Tasrina Rabia Choudhury G. Abdulkreem-Alsultan Shahjalal Khandaker Md. Rabiul Awual
author_facet	Aminul Islam Srimonta Roy Masud Ali Khan Pronoy Mondal Teo, Siow Hwa Yap, Taufiq Yun Hin Mohammad Tofayal Ahmed Tasrina Rabia Choudhury G. Abdulkreem-Alsultan Shahjalal Khandaker Md. Rabiul Awual
author_sort	Aminul Islam
title	Improving valuable metal ions capturing from spent Li-ion batteries with novel materials and approaches
title_short	Improving valuable metal ions capturing from spent Li-ion batteries with novel materials and approaches
title_full	Improving valuable metal ions capturing from spent Li-ion batteries with novel materials and approaches
title_fullStr	Improving valuable metal ions capturing from spent Li-ion batteries with novel materials and approaches
title_full_unstemmed	Improving valuable metal ions capturing from spent Li-ion batteries with novel materials and approaches
title_sort	improving valuable metal ions capturing from spent li-ion batteries with novel materials and approaches
publisher	Elsevier
publishDate	2021
url	https://eprints.ums.edu.my/id/eprint/30349/1/Improving%20valuable%20metal%20ions%20capturing%20from%20spent%20Li-ion%20batteries%20with%20novel%20materials%20and%20approaches%20ABSTRACT.pdf https://eprints.ums.edu.my/id/eprint/30349/2/Improving%20valuable%20metal%20ions%20capturing%20from%20spent%20Li-ion%20batteries%20with%20novel%20materials%20and%20approaches%20FULL%20TEXT.pdf https://eprints.ums.edu.my/id/eprint/30349/ https://www.sciencedirect.com/science/article/pii/S0167732221014276?casa_token=tS4uEg5pR0IAAAAA:SHd4z1kST8tk1OipFqfdVnXAYaV3zGV0DOuMm_yqIn42Cqup6l4tk1eqmJFcTHdAsOnKyCXhtOzQ https://doi.org/10.1016/j.molliq.2021.116703
_version_	1760230751760023552
score	13.211869

Improving valuable metal ions capturing from spent Li-ion batteries with novel materials and approaches

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