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Unveiling the effects of nickel loading on methane dry reforming: Perspectives from Ni/fibrous Zeolite-Y catalysts

The development of new technologies that employ greenhouse gases, such as CO2 and CH4, is becoming more important in the fight against global warming. Catalytic methane dry reforming (MDR) is one straightforward way to reduce CO2 and CH4. In this study, the influence of nickel (Ni) loading on the ca...

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Main Authors: Siti Nurqurratulainie, Miskan, Abdulkadir, Bashir Abubakar, Nurul Aini, Razali, Aishah, Abd Jalil, Lim, Jun Wei, Herma Dina, Setiabudi
Format: Article
Language:English
English
Published: Elsevier Ltd 2024
Subjects:
TP Chemical technology
Online Access:http://umpir.ump.edu.my/id/eprint/41621/1/Unveiling%20the%20effects%20of%20nickel%20loading%20on%20methane%20dry%20reforming_ABST.pdf
http://umpir.ump.edu.my/id/eprint/41621/2/Unveiling%20the%20effects%20of%20nickel%20loading%20on%20methane%20dry%20reforming.pdf
http://umpir.ump.edu.my/id/eprint/41621/
https://doi.org/10.1016/j.ijhydene.2024.05.058
https://doi.org/10.1016/j.ijhydene.2024.05.058
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spelling my.ump.umpir.416212024-07-03T03:51:17Z http://umpir.ump.edu.my/id/eprint/41621/ Unveiling the effects of nickel loading on methane dry reforming: Perspectives from Ni/fibrous Zeolite-Y catalysts Siti Nurqurratulainie, Miskan Abdulkadir, Bashir Abubakar Nurul Aini, Razali Aishah, Abd Jalil Lim, Jun Wei Herma Dina, Setiabudi TP Chemical technology The development of new technologies that employ greenhouse gases, such as CO2 and CH4, is becoming more important in the fight against global warming. Catalytic methane dry reforming (MDR) is one straightforward way to reduce CO2 and CH4. In this study, the influence of nickel (Ni) loading on the catalytic performance of fibrous zeolite-Y catalysts (Ni/FHY) for MDR was explored. The study involved the synthesis and testing of Ni/FHY with varying Ni loadings (1 wt% to 10 wt%). The results demonstrate that the metal loading significantly affects the catalysts' performance through metal-support interaction. The catalytic activity showed that the performance of FHY increased with optimum metal loading of 5 wt% where the CO2 conversion increased to 90.3% from 82.2%, and CH4 conversion to 94.2% from 79.6%. The findings suggest that the 5 wt% optimal Ni loading showed the critical role of the metal-support interaction in shaping catalytic properties. Hence, this work provides insights into catalyst optimization for sustainable industrial processes, highlights the importance of the synergistic metal-support interaction, and provides insights into the relationship between Ni content and catalytic behavior. Thus, it offers a basis for optimizing catalysts in MDR and contributes to the advancement of sustainable industrial processes. Elsevier Ltd 2024-05-14 Article PeerReviewed pdf en http://umpir.ump.edu.my/id/eprint/41621/1/Unveiling%20the%20effects%20of%20nickel%20loading%20on%20methane%20dry%20reforming_ABST.pdf pdf en http://umpir.ump.edu.my/id/eprint/41621/2/Unveiling%20the%20effects%20of%20nickel%20loading%20on%20methane%20dry%20reforming.pdf Siti Nurqurratulainie, Miskan and Abdulkadir, Bashir Abubakar and Nurul Aini, Razali and Aishah, Abd Jalil and Lim, Jun Wei and Herma Dina, Setiabudi (2024) Unveiling the effects of nickel loading on methane dry reforming: Perspectives from Ni/fibrous Zeolite-Y catalysts. International Journal of Hydrogen Energy. pp. 1-11. ISSN 0360-3199. (In Press / Online First) (In Press / Online First) https://doi.org/10.1016/j.ijhydene.2024.05.058 https://doi.org/10.1016/j.ijhydene.2024.05.058
institution Universiti Malaysia Pahang Al-Sultan Abdullah
building UMPSA Library
collection Institutional Repository
continent Asia
country Malaysia
content_provider Universiti Malaysia Pahang Al-Sultan Abdullah
content_source UMPSA Institutional Repository
url_provider http://umpir.ump.edu.my/
language English
English
topic TP Chemical technology
spellingShingle TP Chemical technology
Siti Nurqurratulainie, Miskan
Abdulkadir, Bashir Abubakar
Nurul Aini, Razali
Aishah, Abd Jalil
Lim, Jun Wei
Herma Dina, Setiabudi
Unveiling the effects of nickel loading on methane dry reforming: Perspectives from Ni/fibrous Zeolite-Y catalysts
description The development of new technologies that employ greenhouse gases, such as CO2 and CH4, is becoming more important in the fight against global warming. Catalytic methane dry reforming (MDR) is one straightforward way to reduce CO2 and CH4. In this study, the influence of nickel (Ni) loading on the catalytic performance of fibrous zeolite-Y catalysts (Ni/FHY) for MDR was explored. The study involved the synthesis and testing of Ni/FHY with varying Ni loadings (1 wt% to 10 wt%). The results demonstrate that the metal loading significantly affects the catalysts' performance through metal-support interaction. The catalytic activity showed that the performance of FHY increased with optimum metal loading of 5 wt% where the CO2 conversion increased to 90.3% from 82.2%, and CH4 conversion to 94.2% from 79.6%. The findings suggest that the 5 wt% optimal Ni loading showed the critical role of the metal-support interaction in shaping catalytic properties. Hence, this work provides insights into catalyst optimization for sustainable industrial processes, highlights the importance of the synergistic metal-support interaction, and provides insights into the relationship between Ni content and catalytic behavior. Thus, it offers a basis for optimizing catalysts in MDR and contributes to the advancement of sustainable industrial processes.
format Article
author Siti Nurqurratulainie, Miskan
Abdulkadir, Bashir Abubakar
Nurul Aini, Razali
Aishah, Abd Jalil
Lim, Jun Wei
Herma Dina, Setiabudi
author_facet Siti Nurqurratulainie, Miskan
Abdulkadir, Bashir Abubakar
Nurul Aini, Razali
Aishah, Abd Jalil
Lim, Jun Wei
Herma Dina, Setiabudi
author_sort Siti Nurqurratulainie, Miskan
title Unveiling the effects of nickel loading on methane dry reforming: Perspectives from Ni/fibrous Zeolite-Y catalysts
title_short Unveiling the effects of nickel loading on methane dry reforming: Perspectives from Ni/fibrous Zeolite-Y catalysts
title_full Unveiling the effects of nickel loading on methane dry reforming: Perspectives from Ni/fibrous Zeolite-Y catalysts
title_fullStr Unveiling the effects of nickel loading on methane dry reforming: Perspectives from Ni/fibrous Zeolite-Y catalysts
title_full_unstemmed Unveiling the effects of nickel loading on methane dry reforming: Perspectives from Ni/fibrous Zeolite-Y catalysts
title_sort unveiling the effects of nickel loading on methane dry reforming: perspectives from ni/fibrous zeolite-y catalysts
publisher Elsevier Ltd
publishDate 2024
url http://umpir.ump.edu.my/id/eprint/41621/1/Unveiling%20the%20effects%20of%20nickel%20loading%20on%20methane%20dry%20reforming_ABST.pdf
http://umpir.ump.edu.my/id/eprint/41621/2/Unveiling%20the%20effects%20of%20nickel%20loading%20on%20methane%20dry%20reforming.pdf
http://umpir.ump.edu.my/id/eprint/41621/
https://doi.org/10.1016/j.ijhydene.2024.05.058
https://doi.org/10.1016/j.ijhydene.2024.05.058
_version_ 1822924440390860800
score 13.235796

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