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Facile synthesis of fibrous Faujasite Y supported Ni (Ni/FFY) catalyst for hydrogen production via glycerol dry reforming

In this study, the dendritic structure of Ni-supported Fibrous Faujasite Y (Ni/FFY) catalyst was successfully synthesized by employing a hydrothermal-assisted microemulsion system and subsequently tested in glycerol dry reforming to produce syngas. FFY possesses high porosity due to the formation of...

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Main Authors: Nornasuha, Abdullah, Nurul Aini, Razali, Herma Dina, Setiabudi, Asmida, Ideris, A. R., Mohamed, A. A., Jalil
Format: Article
Language:English
English
Published: Elsevier Ltd 2023
Subjects:
TP Chemical technology
Online Access:http://umpir.ump.edu.my/id/eprint/40532/1/Facile%20synthesis%20of%20fibrous%20Faujasite%20Y%20supported%20Ni.pdf
http://umpir.ump.edu.my/id/eprint/40532/2/Facile%20synthesis%20of%20fibrous%20Faujasite%20Y%20supported%20Ni_FULL.pdf
http://umpir.ump.edu.my/id/eprint/40532/
https://doi.org/10.1016/j.matpr.2023.06.314
https://doi.org/10.1016/j.matpr.2023.06.314
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spelling my.ump.umpir.405322024-02-28T06:55:02Z http://umpir.ump.edu.my/id/eprint/40532/ Facile synthesis of fibrous Faujasite Y supported Ni (Ni/FFY) catalyst for hydrogen production via glycerol dry reforming Nornasuha, Abdullah Nurul Aini, Razali Herma Dina, Setiabudi Asmida, Ideris A. R., Mohamed A. A., Jalil TP Chemical technology In this study, the dendritic structure of Ni-supported Fibrous Faujasite Y (Ni/FFY) catalyst was successfully synthesized by employing a hydrothermal-assisted microemulsion system and subsequently tested in glycerol dry reforming to produce syngas. FFY possesses high porosity due to the formation of radial wrinkle fibre observed from TEM analysis. This provides a huge amount of interparticle pores that facilitate the absorption of the molecules within the material under a minimum hindrance, hence boosting the interior surface accessibility of Ni/FFY. This exclusive morphology contributed to the enhancement in the amount of accessible Ni active sites, resulting in the good activity of Ni/FFY (C3H8O3 conversion = 56.28 %, CO yield = 70.14 %, and H2 yield = 49.80 %). The extraordinary physicochemical properties of Ni/FFY and outstanding catalytic performance in glycerol dry reforming proved its capability as a sustainable catalyst in transforming waste byproduct (glycerol) and greenhouse gas (CO2) to clean energy (H2). This finding presents a pioneering fibrous zeolite catalyst for hydrogen generation in glycerol reforming. Elsevier Ltd 2023-07 Article PeerReviewed pdf en http://umpir.ump.edu.my/id/eprint/40532/1/Facile%20synthesis%20of%20fibrous%20Faujasite%20Y%20supported%20Ni.pdf pdf en http://umpir.ump.edu.my/id/eprint/40532/2/Facile%20synthesis%20of%20fibrous%20Faujasite%20Y%20supported%20Ni_FULL.pdf Nornasuha, Abdullah and Nurul Aini, Razali and Herma Dina, Setiabudi and Asmida, Ideris and A. R., Mohamed and A. A., Jalil (2023) Facile synthesis of fibrous Faujasite Y supported Ni (Ni/FFY) catalyst for hydrogen production via glycerol dry reforming. Materials Today: Proceedings. pp. 1-7. ISSN 2214-7853. (In Press / Online First) (In Press / Online First) https://doi.org/10.1016/j.matpr.2023.06.314 https://doi.org/10.1016/j.matpr.2023.06.314
institution Universiti Malaysia Pahang Al-Sultan Abdullah
building UMPSA Library
collection Institutional Repository
continent Asia
country Malaysia
content_provider Universiti Malaysia Pahang Al-Sultan Abdullah
content_source UMPSA Institutional Repository
url_provider http://umpir.ump.edu.my/
language English
English
topic TP Chemical technology
spellingShingle TP Chemical technology
Nornasuha, Abdullah
Nurul Aini, Razali
Herma Dina, Setiabudi
Asmida, Ideris
A. R., Mohamed
A. A., Jalil
Facile synthesis of fibrous Faujasite Y supported Ni (Ni/FFY) catalyst for hydrogen production via glycerol dry reforming
description In this study, the dendritic structure of Ni-supported Fibrous Faujasite Y (Ni/FFY) catalyst was successfully synthesized by employing a hydrothermal-assisted microemulsion system and subsequently tested in glycerol dry reforming to produce syngas. FFY possesses high porosity due to the formation of radial wrinkle fibre observed from TEM analysis. This provides a huge amount of interparticle pores that facilitate the absorption of the molecules within the material under a minimum hindrance, hence boosting the interior surface accessibility of Ni/FFY. This exclusive morphology contributed to the enhancement in the amount of accessible Ni active sites, resulting in the good activity of Ni/FFY (C3H8O3 conversion = 56.28 %, CO yield = 70.14 %, and H2 yield = 49.80 %). The extraordinary physicochemical properties of Ni/FFY and outstanding catalytic performance in glycerol dry reforming proved its capability as a sustainable catalyst in transforming waste byproduct (glycerol) and greenhouse gas (CO2) to clean energy (H2). This finding presents a pioneering fibrous zeolite catalyst for hydrogen generation in glycerol reforming.
format Article
author Nornasuha, Abdullah
Nurul Aini, Razali
Herma Dina, Setiabudi
Asmida, Ideris
A. R., Mohamed
A. A., Jalil
author_facet Nornasuha, Abdullah
Nurul Aini, Razali
Herma Dina, Setiabudi
Asmida, Ideris
A. R., Mohamed
A. A., Jalil
author_sort Nornasuha, Abdullah
title Facile synthesis of fibrous Faujasite Y supported Ni (Ni/FFY) catalyst for hydrogen production via glycerol dry reforming
title_short Facile synthesis of fibrous Faujasite Y supported Ni (Ni/FFY) catalyst for hydrogen production via glycerol dry reforming
title_full Facile synthesis of fibrous Faujasite Y supported Ni (Ni/FFY) catalyst for hydrogen production via glycerol dry reforming
title_fullStr Facile synthesis of fibrous Faujasite Y supported Ni (Ni/FFY) catalyst for hydrogen production via glycerol dry reforming
title_full_unstemmed Facile synthesis of fibrous Faujasite Y supported Ni (Ni/FFY) catalyst for hydrogen production via glycerol dry reforming
title_sort facile synthesis of fibrous faujasite y supported ni (ni/ffy) catalyst for hydrogen production via glycerol dry reforming
publisher Elsevier Ltd
publishDate 2023
url http://umpir.ump.edu.my/id/eprint/40532/1/Facile%20synthesis%20of%20fibrous%20Faujasite%20Y%20supported%20Ni.pdf
http://umpir.ump.edu.my/id/eprint/40532/2/Facile%20synthesis%20of%20fibrous%20Faujasite%20Y%20supported%20Ni_FULL.pdf
http://umpir.ump.edu.my/id/eprint/40532/
https://doi.org/10.1016/j.matpr.2023.06.314
https://doi.org/10.1016/j.matpr.2023.06.314
_version_ 1822924163624468480
score 13.235796

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