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Hybrid cellulose nanocrystals and graphene oxide polysulfone membranes for copper removal

Polysulfone (PSF) membranes blended with cellulose nanocrystals (CNC) and graphene oxide (GO) nanofiller were prepared for copper removal in this study. The impacts of single CNC, GO, and mixed CNC-GO addition on the morphology, hydrophilicity, permeability, copper ion rejection, and membrane bindin...

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Main Authors:	Siti Nurul Najiah, Abd Rasid, Nor Azura, Che Mahmud, Syed Mohd, Saufi, Takriff, Mohd Sobri, Ang, Wei Lun
Format:	Article
Language:	English
Published:	Desalination Publications 2022
Subjects:	QD Chemistry T Technology (General) TA Engineering (General). Civil engineering (General) TP Chemical technology
Online Access:	http://umpir.ump.edu.my/id/eprint/40188/1/Hybrid%20cellulose%20nanocrystals%20and%20graphene%20oxide%20polysulfone.pdf http://umpir.ump.edu.my/id/eprint/40188/ https://doi.org/10.5004/dwt.2022.28912 https://doi.org/10.5004/dwt.2022.28912
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spelling	my.ump.umpir.401882024-02-08T04:41:13Z http://umpir.ump.edu.my/id/eprint/40188/ Hybrid cellulose nanocrystals and graphene oxide polysulfone membranes for copper removal Siti Nurul Najiah, Abd Rasid Nor Azura, Che Mahmud Syed Mohd, Saufi Takriff, Mohd Sobri Ang, Wei Lun QD Chemistry T Technology (General) TA Engineering (General). Civil engineering (General) TP Chemical technology Polysulfone (PSF) membranes blended with cellulose nanocrystals (CNC) and graphene oxide (GO) nanofiller were prepared for copper removal in this study. The impacts of single CNC, GO, and mixed CNC-GO addition on the morphology, hydrophilicity, permeability, copper ion rejection, and membrane binding capacity were discussed. Scanning electron microscopy results showed that incorporating CNC, GO, and CNC-GO resulted in a more porous membrane structure with a high porosity value. The hydrophilicity of hybrid CNC-GO-PSF membranes were improved with the increment of CNC content and inclusion of the GO filler. Hybrid membranes showed a significant increment of flux compared to pristine PSF membrane. The water flux of the hybrid P-1GO-2C membrane is 8-fold higher than the pure PSF membrane (3.31 L/m2•h). However, the copper rejection of the hybrid CNC-GO-PSF membranes was less than 50%. The increment of the CNC in the hybrid CNC-GO-PSF membrane increases the membrane porosity, and the sub-layer structure of the membrane is becoming very loose. In adsorptive filtration mode, the GO-PSF membrane showed the highest copper binding capacity of 8.49 mg•Cu/g membrane. Desalination Publications 2022-10 Article PeerReviewed pdf en http://umpir.ump.edu.my/id/eprint/40188/1/Hybrid%20cellulose%20nanocrystals%20and%20graphene%20oxide%20polysulfone.pdf Siti Nurul Najiah, Abd Rasid and Nor Azura, Che Mahmud and Syed Mohd, Saufi and Takriff, Mohd Sobri and Ang, Wei Lun (2022) Hybrid cellulose nanocrystals and graphene oxide polysulfone membranes for copper removal. Desalination and Water Treatment, 274. pp. 39-48. ISSN 1944-3994. (Published) https://doi.org/10.5004/dwt.2022.28912 https://doi.org/10.5004/dwt.2022.28912
institution	Universiti Malaysia Pahang Al-Sultan Abdullah
building	UMPSA Library
collection	Institutional Repository
continent	Asia
country	Malaysia
content_provider	Universiti Malaysia Pahang Al-Sultan Abdullah
content_source	UMPSA Institutional Repository
url_provider	http://umpir.ump.edu.my/
language	English
topic	QD Chemistry T Technology (General) TA Engineering (General). Civil engineering (General) TP Chemical technology
spellingShingle	QD Chemistry T Technology (General) TA Engineering (General). Civil engineering (General) TP Chemical technology Siti Nurul Najiah, Abd Rasid Nor Azura, Che Mahmud Syed Mohd, Saufi Takriff, Mohd Sobri Ang, Wei Lun Hybrid cellulose nanocrystals and graphene oxide polysulfone membranes for copper removal
description	Polysulfone (PSF) membranes blended with cellulose nanocrystals (CNC) and graphene oxide (GO) nanofiller were prepared for copper removal in this study. The impacts of single CNC, GO, and mixed CNC-GO addition on the morphology, hydrophilicity, permeability, copper ion rejection, and membrane binding capacity were discussed. Scanning electron microscopy results showed that incorporating CNC, GO, and CNC-GO resulted in a more porous membrane structure with a high porosity value. The hydrophilicity of hybrid CNC-GO-PSF membranes were improved with the increment of CNC content and inclusion of the GO filler. Hybrid membranes showed a significant increment of flux compared to pristine PSF membrane. The water flux of the hybrid P-1GO-2C membrane is 8-fold higher than the pure PSF membrane (3.31 L/m2•h). However, the copper rejection of the hybrid CNC-GO-PSF membranes was less than 50%. The increment of the CNC in the hybrid CNC-GO-PSF membrane increases the membrane porosity, and the sub-layer structure of the membrane is becoming very loose. In adsorptive filtration mode, the GO-PSF membrane showed the highest copper binding capacity of 8.49 mg•Cu/g membrane.
format	Article
author	Siti Nurul Najiah, Abd Rasid Nor Azura, Che Mahmud Syed Mohd, Saufi Takriff, Mohd Sobri Ang, Wei Lun
author_facet	Siti Nurul Najiah, Abd Rasid Nor Azura, Che Mahmud Syed Mohd, Saufi Takriff, Mohd Sobri Ang, Wei Lun
author_sort	Siti Nurul Najiah, Abd Rasid
title	Hybrid cellulose nanocrystals and graphene oxide polysulfone membranes for copper removal
title_short	Hybrid cellulose nanocrystals and graphene oxide polysulfone membranes for copper removal
title_full	Hybrid cellulose nanocrystals and graphene oxide polysulfone membranes for copper removal
title_fullStr	Hybrid cellulose nanocrystals and graphene oxide polysulfone membranes for copper removal
title_full_unstemmed	Hybrid cellulose nanocrystals and graphene oxide polysulfone membranes for copper removal
title_sort	hybrid cellulose nanocrystals and graphene oxide polysulfone membranes for copper removal
publisher	Desalination Publications
publishDate	2022
url	http://umpir.ump.edu.my/id/eprint/40188/1/Hybrid%20cellulose%20nanocrystals%20and%20graphene%20oxide%20polysulfone.pdf http://umpir.ump.edu.my/id/eprint/40188/ https://doi.org/10.5004/dwt.2022.28912 https://doi.org/10.5004/dwt.2022.28912
_version_	1822924123533213696
score	13.232414

Hybrid cellulose nanocrystals and graphene oxide polysulfone membranes for copper removal

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