Properties-activity correlation of Nickel supported on fibrous Zeolite-Y for dry reforming of methane

Nickel-supported Fibrous zeolite-Y (Ni/FHY) was successfully synthesized via the microemulsion method using HY as seed, followed by catalytic evaluation in dry reforming of methane (DRM) for hydrogen production. Ni/FHY possessed good NiO distribution, improved metal-support interface, and strong bas...

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Main Authors: S.N., Miskan, H.D., Setiabudi, M.B., Bahari, Vo, Dai-Viet N., B., Abdullah, A.A., Jalil, S.A.F., Syed Muhammad, S.B., Ismail
Format: Article
Language:English
English
Published: Elsevier Ltd 2023
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Online Access:http://umpir.ump.edu.my/id/eprint/39200/1/Properties-activity%20correlation%20of%20Nickel%20supported.pdf
http://umpir.ump.edu.my/id/eprint/39200/2/Properties-activity%20correlation%20of%20Nickel%20supported%20on%20fibrous%20zeolite-y%20for%20dry%20reforming%20of%20methane.pdf
http://umpir.ump.edu.my/id/eprint/39200/
https://doi.org/10.1016/j.ijhydene.2022.12.201
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spelling my.ump.umpir.392002023-11-08T00:54:14Z http://umpir.ump.edu.my/id/eprint/39200/ Properties-activity correlation of Nickel supported on fibrous Zeolite-Y for dry reforming of methane S.N., Miskan H.D., Setiabudi M.B., Bahari Vo, Dai-Viet N. B., Abdullah A.A., Jalil S.A.F., Syed Muhammad S.B., Ismail T Technology (General) TP Chemical technology Nickel-supported Fibrous zeolite-Y (Ni/FHY) was successfully synthesized via the microemulsion method using HY as seed, followed by catalytic evaluation in dry reforming of methane (DRM) for hydrogen production. Ni/FHY possessed good NiO distribution, improved metal-support interface, and strong basicity, accredited to the fibrous structure of FHY. This unique morphology led to the enrichment in the amount of accessible Ni active sites, thus resulting in the superior activity of Ni/FHY (XCH=95.1%,XCO=91.1%,H2/CO=0.89) compared to Ni/HY (XCH=92.7%,XCO=89.8%,H2/CO=0.78). Meanwhile, the inferior performance of Ni/HY could be caused by the poor distribution of Ni with large particles, thus contributing to high carbon deposition and Ni sintering. The unique physicochemical properties and superior catalytic activity confirmed its viability in the DRM. Elsevier Ltd 2023 Article PeerReviewed pdf en http://umpir.ump.edu.my/id/eprint/39200/1/Properties-activity%20correlation%20of%20Nickel%20supported.pdf pdf en http://umpir.ump.edu.my/id/eprint/39200/2/Properties-activity%20correlation%20of%20Nickel%20supported%20on%20fibrous%20zeolite-y%20for%20dry%20reforming%20of%20methane.pdf S.N., Miskan and H.D., Setiabudi and M.B., Bahari and Vo, Dai-Viet N. and B., Abdullah and A.A., Jalil and S.A.F., Syed Muhammad and S.B., Ismail (2023) Properties-activity correlation of Nickel supported on fibrous Zeolite-Y for dry reforming of methane. International Journal of Hydrogen Energy. ISSN 0360-3199. (In Press / Online First) (In Press / Online First) https://doi.org/10.1016/j.ijhydene.2022.12.201 10.1016/j.ijhydene.2022.12.201
institution Universiti Malaysia Pahang Al-Sultan Abdullah
building UMPSA Library
collection Institutional Repository
continent Asia
country Malaysia
content_provider Universiti Malaysia Pahang Al-Sultan Abdullah
content_source UMPSA Institutional Repository
url_provider http://umpir.ump.edu.my/
language English
English
topic T Technology (General)
TP Chemical technology
spellingShingle T Technology (General)
TP Chemical technology
S.N., Miskan
H.D., Setiabudi
M.B., Bahari
Vo, Dai-Viet N.
B., Abdullah
A.A., Jalil
S.A.F., Syed Muhammad
S.B., Ismail
Properties-activity correlation of Nickel supported on fibrous Zeolite-Y for dry reforming of methane
description Nickel-supported Fibrous zeolite-Y (Ni/FHY) was successfully synthesized via the microemulsion method using HY as seed, followed by catalytic evaluation in dry reforming of methane (DRM) for hydrogen production. Ni/FHY possessed good NiO distribution, improved metal-support interface, and strong basicity, accredited to the fibrous structure of FHY. This unique morphology led to the enrichment in the amount of accessible Ni active sites, thus resulting in the superior activity of Ni/FHY (XCH=95.1%,XCO=91.1%,H2/CO=0.89) compared to Ni/HY (XCH=92.7%,XCO=89.8%,H2/CO=0.78). Meanwhile, the inferior performance of Ni/HY could be caused by the poor distribution of Ni with large particles, thus contributing to high carbon deposition and Ni sintering. The unique physicochemical properties and superior catalytic activity confirmed its viability in the DRM.
format Article
author S.N., Miskan
H.D., Setiabudi
M.B., Bahari
Vo, Dai-Viet N.
B., Abdullah
A.A., Jalil
S.A.F., Syed Muhammad
S.B., Ismail
author_facet S.N., Miskan
H.D., Setiabudi
M.B., Bahari
Vo, Dai-Viet N.
B., Abdullah
A.A., Jalil
S.A.F., Syed Muhammad
S.B., Ismail
author_sort S.N., Miskan
title Properties-activity correlation of Nickel supported on fibrous Zeolite-Y for dry reforming of methane
title_short Properties-activity correlation of Nickel supported on fibrous Zeolite-Y for dry reforming of methane
title_full Properties-activity correlation of Nickel supported on fibrous Zeolite-Y for dry reforming of methane
title_fullStr Properties-activity correlation of Nickel supported on fibrous Zeolite-Y for dry reforming of methane
title_full_unstemmed Properties-activity correlation of Nickel supported on fibrous Zeolite-Y for dry reforming of methane
title_sort properties-activity correlation of nickel supported on fibrous zeolite-y for dry reforming of methane
publisher Elsevier Ltd
publishDate 2023
url http://umpir.ump.edu.my/id/eprint/39200/1/Properties-activity%20correlation%20of%20Nickel%20supported.pdf
http://umpir.ump.edu.my/id/eprint/39200/2/Properties-activity%20correlation%20of%20Nickel%20supported%20on%20fibrous%20zeolite-y%20for%20dry%20reforming%20of%20methane.pdf
http://umpir.ump.edu.my/id/eprint/39200/
https://doi.org/10.1016/j.ijhydene.2022.12.201
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