Multi-dimensional dynamic fluorescence readout from laser engineered In2O3 nanowire micropatterns

Laser-induced microscale reactions are an excellent means to obtain controllable, small-scale insights into nanomaterial properties. Importantly, the opportunity for a comprehensive understanding of the material's optical origins allows for refined engineering of material luminescence. Modifyin...

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Main Authors: Poh, Eng Tuan, Tan, Yung Zhen, Neo, Justin Boon Shuan, Ong, Chee How, Saroni, Azianty, Zhang, Zheng, Li, Jianhui, Goh, Boon Tong, Sow, Chorng Haur
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Published: ROYAL SOC CHEMISTRY 2023
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Online Access:http://eprints.um.edu.my/38287/
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spelling my.um.eprints.382872024-06-15T03:49:49Z http://eprints.um.edu.my/38287/ Multi-dimensional dynamic fluorescence readout from laser engineered In2O3 nanowire micropatterns Poh, Eng Tuan Tan, Yung Zhen Neo, Justin Boon Shuan Ong, Chee How Saroni, Azianty Zhang, Zheng Li, Jianhui Goh, Boon Tong Sow, Chorng Haur QC Physics Laser-induced microscale reactions are an excellent means to obtain controllable, small-scale insights into nanomaterial properties. Importantly, the opportunity for a comprehensive understanding of the material's optical origins allows for refined engineering of material luminescence. Modifying an array of standing indium oxide (In2O3) nanowires with a focused laser beam, we report newfound yellow and blue fluorescence emanating from the sample. Evaluated through a broad range of laser conditions, the laser-induced yellow component was found to relate to oxygen inclusions, while the blue fluorescence overlayer originated from oxygen physisorption upon prolonged storage. Capitalizing on the versatility of the blue emission component under UV modulation, we demonstrate micropatterns with multiple layers of differentiated optical encryption features. The enhanced anti-counterfeiting capability allows improved complexity in an authentication process, involving the convergence of microscale patterning, dynamic color evolution and time-domain encoding as multilevel checkpoints in the verification process. ROYAL SOC CHEMISTRY 2023-04 Article PeerReviewed Poh, Eng Tuan and Tan, Yung Zhen and Neo, Justin Boon Shuan and Ong, Chee How and Saroni, Azianty and Zhang, Zheng and Li, Jianhui and Goh, Boon Tong and Sow, Chorng Haur (2023) Multi-dimensional dynamic fluorescence readout from laser engineered In2O3 nanowire micropatterns. JOURNAL OF MATERIALS CHEMISTRY C, 11 (16). pp. 5271-5280. ISSN 2050-7526, DOI https://doi.org/10.1039/d2tc04449h <https://doi.org/10.1039/d2tc04449h>. 10.1039/d2tc04449h
institution Universiti Malaya
building UM Library
collection Institutional Repository
continent Asia
country Malaysia
content_provider Universiti Malaya
content_source UM Research Repository
url_provider http://eprints.um.edu.my/
topic QC Physics
spellingShingle QC Physics
Poh, Eng Tuan
Tan, Yung Zhen
Neo, Justin Boon Shuan
Ong, Chee How
Saroni, Azianty
Zhang, Zheng
Li, Jianhui
Goh, Boon Tong
Sow, Chorng Haur
Multi-dimensional dynamic fluorescence readout from laser engineered In2O3 nanowire micropatterns
description Laser-induced microscale reactions are an excellent means to obtain controllable, small-scale insights into nanomaterial properties. Importantly, the opportunity for a comprehensive understanding of the material's optical origins allows for refined engineering of material luminescence. Modifying an array of standing indium oxide (In2O3) nanowires with a focused laser beam, we report newfound yellow and blue fluorescence emanating from the sample. Evaluated through a broad range of laser conditions, the laser-induced yellow component was found to relate to oxygen inclusions, while the blue fluorescence overlayer originated from oxygen physisorption upon prolonged storage. Capitalizing on the versatility of the blue emission component under UV modulation, we demonstrate micropatterns with multiple layers of differentiated optical encryption features. The enhanced anti-counterfeiting capability allows improved complexity in an authentication process, involving the convergence of microscale patterning, dynamic color evolution and time-domain encoding as multilevel checkpoints in the verification process.
format Article
author Poh, Eng Tuan
Tan, Yung Zhen
Neo, Justin Boon Shuan
Ong, Chee How
Saroni, Azianty
Zhang, Zheng
Li, Jianhui
Goh, Boon Tong
Sow, Chorng Haur
author_facet Poh, Eng Tuan
Tan, Yung Zhen
Neo, Justin Boon Shuan
Ong, Chee How
Saroni, Azianty
Zhang, Zheng
Li, Jianhui
Goh, Boon Tong
Sow, Chorng Haur
author_sort Poh, Eng Tuan
title Multi-dimensional dynamic fluorescence readout from laser engineered In2O3 nanowire micropatterns
title_short Multi-dimensional dynamic fluorescence readout from laser engineered In2O3 nanowire micropatterns
title_full Multi-dimensional dynamic fluorescence readout from laser engineered In2O3 nanowire micropatterns
title_fullStr Multi-dimensional dynamic fluorescence readout from laser engineered In2O3 nanowire micropatterns
title_full_unstemmed Multi-dimensional dynamic fluorescence readout from laser engineered In2O3 nanowire micropatterns
title_sort multi-dimensional dynamic fluorescence readout from laser engineered in2o3 nanowire micropatterns
publisher ROYAL SOC CHEMISTRY
publishDate 2023
url http://eprints.um.edu.my/38287/
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score 13.211869