Multi-dimensional dynamic fluorescence readout from laser engineered In2O3 nanowire micropatterns
Laser-induced microscale reactions are an excellent means to obtain controllable, small-scale insights into nanomaterial properties. Importantly, the opportunity for a comprehensive understanding of the material's optical origins allows for refined engineering of material luminescence. Modifyin...
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ROYAL SOC CHEMISTRY
2023
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my.um.eprints.382872024-06-15T03:49:49Z http://eprints.um.edu.my/38287/ Multi-dimensional dynamic fluorescence readout from laser engineered In2O3 nanowire micropatterns Poh, Eng Tuan Tan, Yung Zhen Neo, Justin Boon Shuan Ong, Chee How Saroni, Azianty Zhang, Zheng Li, Jianhui Goh, Boon Tong Sow, Chorng Haur QC Physics Laser-induced microscale reactions are an excellent means to obtain controllable, small-scale insights into nanomaterial properties. Importantly, the opportunity for a comprehensive understanding of the material's optical origins allows for refined engineering of material luminescence. Modifying an array of standing indium oxide (In2O3) nanowires with a focused laser beam, we report newfound yellow and blue fluorescence emanating from the sample. Evaluated through a broad range of laser conditions, the laser-induced yellow component was found to relate to oxygen inclusions, while the blue fluorescence overlayer originated from oxygen physisorption upon prolonged storage. Capitalizing on the versatility of the blue emission component under UV modulation, we demonstrate micropatterns with multiple layers of differentiated optical encryption features. The enhanced anti-counterfeiting capability allows improved complexity in an authentication process, involving the convergence of microscale patterning, dynamic color evolution and time-domain encoding as multilevel checkpoints in the verification process. ROYAL SOC CHEMISTRY 2023-04 Article PeerReviewed Poh, Eng Tuan and Tan, Yung Zhen and Neo, Justin Boon Shuan and Ong, Chee How and Saroni, Azianty and Zhang, Zheng and Li, Jianhui and Goh, Boon Tong and Sow, Chorng Haur (2023) Multi-dimensional dynamic fluorescence readout from laser engineered In2O3 nanowire micropatterns. JOURNAL OF MATERIALS CHEMISTRY C, 11 (16). pp. 5271-5280. ISSN 2050-7526, DOI https://doi.org/10.1039/d2tc04449h <https://doi.org/10.1039/d2tc04449h>. 10.1039/d2tc04449h |
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QC Physics Poh, Eng Tuan Tan, Yung Zhen Neo, Justin Boon Shuan Ong, Chee How Saroni, Azianty Zhang, Zheng Li, Jianhui Goh, Boon Tong Sow, Chorng Haur Multi-dimensional dynamic fluorescence readout from laser engineered In2O3 nanowire micropatterns |
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Laser-induced microscale reactions are an excellent means to obtain controllable, small-scale insights into nanomaterial properties. Importantly, the opportunity for a comprehensive understanding of the material's optical origins allows for refined engineering of material luminescence. Modifying an array of standing indium oxide (In2O3) nanowires with a focused laser beam, we report newfound yellow and blue fluorescence emanating from the sample. Evaluated through a broad range of laser conditions, the laser-induced yellow component was found to relate to oxygen inclusions, while the blue fluorescence overlayer originated from oxygen physisorption upon prolonged storage. Capitalizing on the versatility of the blue emission component under UV modulation, we demonstrate micropatterns with multiple layers of differentiated optical encryption features. The enhanced anti-counterfeiting capability allows improved complexity in an authentication process, involving the convergence of microscale patterning, dynamic color evolution and time-domain encoding as multilevel checkpoints in the verification process. |
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Article |
author |
Poh, Eng Tuan Tan, Yung Zhen Neo, Justin Boon Shuan Ong, Chee How Saroni, Azianty Zhang, Zheng Li, Jianhui Goh, Boon Tong Sow, Chorng Haur |
author_facet |
Poh, Eng Tuan Tan, Yung Zhen Neo, Justin Boon Shuan Ong, Chee How Saroni, Azianty Zhang, Zheng Li, Jianhui Goh, Boon Tong Sow, Chorng Haur |
author_sort |
Poh, Eng Tuan |
title |
Multi-dimensional dynamic fluorescence readout from laser engineered In2O3 nanowire micropatterns |
title_short |
Multi-dimensional dynamic fluorescence readout from laser engineered In2O3 nanowire micropatterns |
title_full |
Multi-dimensional dynamic fluorescence readout from laser engineered In2O3 nanowire micropatterns |
title_fullStr |
Multi-dimensional dynamic fluorescence readout from laser engineered In2O3 nanowire micropatterns |
title_full_unstemmed |
Multi-dimensional dynamic fluorescence readout from laser engineered In2O3 nanowire micropatterns |
title_sort |
multi-dimensional dynamic fluorescence readout from laser engineered in2o3 nanowire micropatterns |
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ROYAL SOC CHEMISTRY |
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2023 |
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http://eprints.um.edu.my/38287/ |
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1805881103250096128 |
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13.211869 |