Perovskite materials in X-ray detection and imaging: recent progress, challenges, and future prospects
Perovskite materials have attracted significant attention as innovative and efficient X-ray detectors owing to their unique properties compared to traditional X-ray detectors. Herein, chronologically, we present an in-depth analysis of X-ray detection technologies employing organic-inorganic hybrids...
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Royal Society of Chemistry
2025
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| author | Miah M.H. Khandaker M.U. Aminul Islam M. Nur-E-Alam M. Osman H. Ullah M.H. |
| author2 | 57373098800 |
| author_facet | 57373098800 Miah M.H. Khandaker M.U. Aminul Islam M. Nur-E-Alam M. Osman H. Ullah M.H. |
| author_sort | Miah M.H. |
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| collection | Institutional Repository |
| content_provider | Universiti Tenaga Nasional |
| content_source | UNITEN Institutional Repository |
| continent | Asia |
| country | Malaysia |
| description | Perovskite materials have attracted significant attention as innovative and efficient X-ray detectors owing to their unique properties compared to traditional X-ray detectors. Herein, chronologically, we present an in-depth analysis of X-ray detection technologies employing organic-inorganic hybrids (OIHs), all-inorganic and lead-free perovskite material-based single crystals (SCs), thin/thick films and wafers. Particularly, this review systematically scrutinizes the advancement of the diverse synthesis methods, structural modifications, and device architectures exploited to enhance the radiation sensing performance. In addition, a critical analysis of the crucial factors affecting the performance of the devices is also provided. Our findings revealed that the improvement from single crystallization techniques dominated the film and wafer growth techniques. The probable reason for this is that SC-based devices display a lower trap density, higher resistivity, large carrier mobility and lifetime compared to film- and wafer-based devices. Ultimately, devices with SCs showed outstanding sensitivity and the lowest detectable dose rate (LDDR). These results are superior to some traditional X-ray detectors such as amorphous selenium and CZT. In addition, the limited performance of film-based devices is attributed to the defect formation in the bulk film, surfaces, and grain boundaries. However, wafer-based devices showed the worst performance because of the formation of voids, which impede the movement of charge carriers. We also observed that by performing structural modification, various research groups achieved high-performance devices together with stability. Finally, by fusing the findings from diverse research works, we provide a valuable resource for researchers in the field of X-ray detection, imaging and materials science. Ultimately, this review will serve as a roadmap for directing the difficulties associated with perovskite materials in X-ray detection and imaging, proposing insights into the recent status, challenges, and promising directions for future research. ? 2024 The Royal Society of Chemistry |
| format | Review |
| id | my.uniten.dspace-36812 |
| institution | Universiti Tenaga Nasional |
| publishDate | 2025 |
| publisher | Royal Society of Chemistry |
| record_format | dspace |
| spelling | my.uniten.dspace-368122025-03-03T15:44:52Z Perovskite materials in X-ray detection and imaging: recent progress, challenges, and future prospects Miah M.H. Khandaker M.U. Aminul Islam M. Nur-E-Alam M. Osman H. Ullah M.H. 57373098800 36836773700 57828419400 57197752581 57222091164 57951098200 Chemical detection Display devices Grain boundaries Organic-inorganic materials Perovskite Single crystals Thin films Detection technology Future prospects In-depth analysis Performance Property Recent progress Structural modifications Wafer-based devices X-ray detections X-ray detector X ray detectors Perovskite materials have attracted significant attention as innovative and efficient X-ray detectors owing to their unique properties compared to traditional X-ray detectors. Herein, chronologically, we present an in-depth analysis of X-ray detection technologies employing organic-inorganic hybrids (OIHs), all-inorganic and lead-free perovskite material-based single crystals (SCs), thin/thick films and wafers. Particularly, this review systematically scrutinizes the advancement of the diverse synthesis methods, structural modifications, and device architectures exploited to enhance the radiation sensing performance. In addition, a critical analysis of the crucial factors affecting the performance of the devices is also provided. Our findings revealed that the improvement from single crystallization techniques dominated the film and wafer growth techniques. The probable reason for this is that SC-based devices display a lower trap density, higher resistivity, large carrier mobility and lifetime compared to film- and wafer-based devices. Ultimately, devices with SCs showed outstanding sensitivity and the lowest detectable dose rate (LDDR). These results are superior to some traditional X-ray detectors such as amorphous selenium and CZT. In addition, the limited performance of film-based devices is attributed to the defect formation in the bulk film, surfaces, and grain boundaries. However, wafer-based devices showed the worst performance because of the formation of voids, which impede the movement of charge carriers. We also observed that by performing structural modification, various research groups achieved high-performance devices together with stability. Finally, by fusing the findings from diverse research works, we provide a valuable resource for researchers in the field of X-ray detection, imaging and materials science. Ultimately, this review will serve as a roadmap for directing the difficulties associated with perovskite materials in X-ray detection and imaging, proposing insights into the recent status, challenges, and promising directions for future research. ? 2024 The Royal Society of Chemistry Final 2025-03-03T07:44:51Z 2025-03-03T07:44:51Z 2024 Review 10.1039/d4ra00433g 2-s2.0-85185881143 https://www.scopus.com/inward/record.uri?eid=2-s2.0-85185881143&doi=10.1039%2fd4ra00433g&partnerID=40&md5=d9efcc35026189892648554f0d2ab8bc https://irepository.uniten.edu.my/handle/123456789/36812 14 10 6656 6698 All Open Access; Gold Open Access; Green Open Access Royal Society of Chemistry Scopus |
| spellingShingle | Chemical detection Display devices Grain boundaries Organic-inorganic materials Perovskite Single crystals Thin films Detection technology Future prospects In-depth analysis Performance Property Recent progress Structural modifications Wafer-based devices X-ray detections X-ray detector X ray detectors Miah M.H. Khandaker M.U. Aminul Islam M. Nur-E-Alam M. Osman H. Ullah M.H. Perovskite materials in X-ray detection and imaging: recent progress, challenges, and future prospects |
| title | Perovskite materials in X-ray detection and imaging: recent progress, challenges, and future prospects |
| title_full | Perovskite materials in X-ray detection and imaging: recent progress, challenges, and future prospects |
| title_fullStr | Perovskite materials in X-ray detection and imaging: recent progress, challenges, and future prospects |
| title_full_unstemmed | Perovskite materials in X-ray detection and imaging: recent progress, challenges, and future prospects |
| title_short | Perovskite materials in X-ray detection and imaging: recent progress, challenges, and future prospects |
| title_sort | perovskite materials in x-ray detection and imaging: recent progress, challenges, and future prospects |
| topic | Chemical detection Display devices Grain boundaries Organic-inorganic materials Perovskite Single crystals Thin films Detection technology Future prospects In-depth analysis Performance Property Recent progress Structural modifications Wafer-based devices X-ray detections X-ray detector X ray detectors |
| url_provider | http://dspace.uniten.edu.my/ |