Coexistence of dielectric relaxation and magnetic relaxation in compressively strained BiFeO3/Ba0.7Sr0.3TiO3 superlattices
Superlattices (SLs) consisting of multiferroic BiFeO3 (BFO) and dielectric Ba0.7Sr0.3TiO3 were epitaxially grown on a (001)-oriented Nb:SrTiO3 substrate using pulsed laser deposition. An improved ferroelectricity with a high-temperature polarization of ∼63.7 μC/cm2 at 470 K was observed. The SL exhi...
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| Main Authors: | , , , , , , , |
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| Format: | Article |
| Published: |
AIP Publishing
2019
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| Subjects: | |
| Online Access: | http://eprints.um.edu.my/16688/ https://doi.org/10.1063/1.5085350 |
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| Summary: | Superlattices (SLs) consisting of multiferroic BiFeO3 (BFO) and dielectric Ba0.7Sr0.3TiO3 were epitaxially grown on a (001)-oriented Nb:SrTiO3 substrate using pulsed laser deposition. An improved ferroelectricity with a high-temperature polarization of ∼63.7 μC/cm2 at 470 K was observed. The SL exhibited both dielectric and magnetic relaxation properties. Two distinct dielectric relaxations were found: a carrier hopping process between Fe2+ and Fe3+ from 273 to 410 K and the long-range migration of oxygen vacancies from 430 to 573 K. Spin-glass behavior with a freezing temperature of ∼86.6 K was also observed. This work provides a promising path forward to tailor the multiferroic properties of BFO-based structures for high-temperature applications. © 2019 Author(s). |
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